I was going to build a 900ltr thermal store for our place, but then our heat source is solid fuel, so the capacity is more useful.
I stopped the idea, not as i thought it wouldnt be good, but simply as i picked up a 300ltr store off ebay for a ton, and it seemed simpler (and more efficient on space) to install that.
Ill build a large one at the next hose, when we have more space and / or motivation. (ie im keeping all the copper coils i had set asside for it - it took me about 18 months to buy them all, so im not loosing them that quick!)
If you have an on/off heat source, then i cant see much point in having a huge store. However, if you did go the glog route, then the larger the better, i think.